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High-resolution spectra of 2ν(OH) overtone of trans-formic acid in the supersonic jet

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F22%3A00562535" target="_blank" >RIV/61388955:_____/22:00562535 - isvavai.cz</a>

  • Result on the web

    <a href="https://hdl.handle.net/11104/0334847" target="_blank" >https://hdl.handle.net/11104/0334847</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.jqsrt.2022.108319" target="_blank" >10.1016/j.jqsrt.2022.108319</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    High-resolution spectra of 2ν(OH) overtone of trans-formic acid in the supersonic jet

  • Original language description

    First high-resolution low-temperature spectrum of the 2ν(OH) overtone of trans-formic acid have been measured using direct-absorption laser spectroscopy. The supersonic cooling in the jet expansion to 37 K has dramatically simplified the complex ro-vibrational structure of the band due to the thermal depopulation of higher-lying rotational states. Altogether, 597 lines have been measured with a line-position accuracy better than 0.001 cm1, and 441 of them have been reliably assigned using a custom-build program for a line-by-line assignment using the ground state combination differences. In total, 39 low-lying upper rota-tional states of the overtone vibration have been calculated from these line assignments. Moreover, some additional states have been also identified and tentatively assigned to a bath of dark states present in this spectral region. A global fit using A-reduced Watson's type Hamiltonian in Ir representation has been per-formed to obtain several ro-vibrational constants for the 2 nu(OH) vibration. In addition, the fit demonstrates the effect of numerous perturbations in the rotational structure.(c) 2022 Elsevier Ltd. All rights reserved.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

    <a href="/en/project/GA19-14105S" target="_blank" >GA19-14105S: Heterogeneous reactions of the atmospheric radicals on clusters.</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2022

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Quantitative Spectroscopy and Radiative Transfer

  • ISSN

    0022-4073

  • e-ISSN

    1879-1352

  • Volume of the periodical

    292

  • Issue of the periodical within the volume

    DEC 2022

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    7

  • Pages from-to

    108319

  • UT code for WoS article

    000862275300002

  • EID of the result in the Scopus database

    2-s2.0-85137170773