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Vibrational excitation in the e + CO2 system: Analysis of the two-dimensional energy-loss spectrum

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F22%3A00566830" target="_blank" >RIV/61388955:_____/22:00566830 - isvavai.cz</a>

  • Alternative codes found

    RIV/00216208:11320/22:10456308

  • Result on the web

    <a href="https://doi.org/10.1103/PhysRevA.106.062807" target="_blank" >https://doi.org/10.1103/PhysRevA.106.062807</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1103/PhysRevA.106.062807" target="_blank" >10.1103/PhysRevA.106.062807</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Vibrational excitation in the e + CO2 system: Analysis of the two-dimensional energy-loss spectrum

  • Original language description

    We present a detailed analysis of the two-dimensional electron energy-loss spectrum of CO2, which extends our recent Letter [Phys. Rev. Lett. 129, 013401 (2022)0031-900710.1103/PhysRevLett.129.013401]. We show that our vibronic coupling model [Phys. Rev. A 105, 062821 (2022)2469-992610.1103/PhysRevA.105.062821] captures primary features of the multidimensional dynamics of the temporary molecular anion, and the calculations qualitatively reproduce the spectrum. The shape of the spectrum is given by two overlapping contributions that originate in excitation of vibrational states within ςg+ and Πu Fermi polyads. Propensity rules in terms of scattered and vibrational wave functions are also discussed to clarify the selectivity of states from the vibrational pseudocontinuum that is responsible for the observed fine structure.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2022

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Physical Review A

  • ISSN

    2469-9926

  • e-ISSN

    2469-9934

  • Volume of the periodical

    106

  • Issue of the periodical within the volume

    6

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    10

  • Pages from-to

    062807

  • UT code for WoS article

    000901724300001

  • EID of the result in the Scopus database

    2-s2.0-85143647594