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Single Molecule Conductance of Anthraquinone-Based Molecular Wire: Effect of the Anchoring Group

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F25%3A00603511" target="_blank" >RIV/61388955:_____/25:00603511 - isvavai.cz</a>

  • Result on the web

    <a href="https://hdl.handle.net/11104/0360841" target="_blank" >https://hdl.handle.net/11104/0360841</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/hlca.202400155" target="_blank" >10.1002/hlca.202400155</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Single Molecule Conductance of Anthraquinone-Based Molecular Wire: Effect of the Anchoring Group

  • Original language description

    Functional molecular electronics require molecular design that provides integrity and stability. In this work, we explored two types of single molecule devices differing in anchoring to the conducting leads. Single molecule conductance was measured by STM break junction method and the molecular conductor was composed of the redox active anthraquinone center (switching element) containing either 4-pyridyl or p-phenylene thioacetate anchoring groups. The experimental results were supported by quantum chemical charge transport calculations. Molecular junctions containing 4-pyridyl anchors displayed two stable configurations with conductance values of 4.9 nS and 20 pS, respectively. Molecules anchored via p-phenylene thioacetate groups led to one main junction configuration with conductance of 0.1 nS. Junctions employing 4-pyridyl anchoring groups had higher junction formation probability, which in combination with lower conductance makes them better candidates for switching purposes.n

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10405 - Electrochemistry (dry cells, batteries, fuel cells, corrosion metals, electrolysis)

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2025

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Helvetica Chimica Acta

  • ISSN

    0018-019X

  • e-ISSN

    1522-2675

  • Volume of the periodical

    108

  • Issue of the periodical within the volume

    2

  • Country of publishing house

    CH - SWITZERLAND

  • Number of pages

    11

  • Pages from-to

    e202400155

  • UT code for WoS article

    001388997500001

  • EID of the result in the Scopus database

    2-s2.0-85214224180