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Gas-phase C-H and N-H bond activation by a high valent nitrido-iron dication and {NH}-transfer to activated olefins

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388963%3A_____%2F08%3A00314403" target="_blank" >RIV/61388963:_____/08:00314403 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    Gas-phase C-H and N-H bond activation by a high valent nitrido-iron dication and {NH}-transfer to activated olefins

  • Original language description

    A tetrapodal pentadentate nitrogen ligand (2,6-bis(1,1-di(aminomethyl)ethyl)pyridine, 1) is used for the synthesis of the azido-iron(III) complex [(1)Fe(N3)]X2 (X =Br or PF6). Electrospray ionization affords the dication [(1)Fe(N3)]2+ as well as the dicationic nitrido-iron species [(1)FeN]2+.

  • Czech name

    Aktivace C-H a N-H vazeb v plynné fázi vysoce valentním dikationtem nitridu kovu a {NH}-přenos k aktivaci olefinů

  • Czech description

    Tetrapodální pentadentální dusíkatý ligand (2,6-bis(1,1-di(aminomethyl)ethyl)pyridine, 1) je používán pro syntézu komplexu azidu kovu(III) [(1)Fe(N3)]X2 (X =Br or PF6). Electrospray ionizace poskytuje dikationt [(1)Fe(N3)]2+ spolu s dikationickými sloučeninami nitridů kovu [(1)FeN]2+.

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/KJB400550704" target="_blank" >KJB400550704: Intrinsic properties of redox-active molecules</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)<br>Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2008

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of the American Chemical Society

  • ISSN

    0002-7863

  • e-ISSN

  • Volume of the periodical

    130

  • Issue of the periodical within the volume

    13

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    10

  • Pages from-to

  • UT code for WoS article

    000254549000028

  • EID of the result in the Scopus database