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Methyl and Pentyl Chloride in a Microhydrated Environment and at the Liquid Water-Vapor Interface: A Theoretical Study

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388963%3A_____%2F11%3A00359024" target="_blank" >RIV/61388963:_____/11:00359024 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1021/jp107989k" target="_blank" >http://dx.doi.org/10.1021/jp107989k</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/jp107989k" target="_blank" >10.1021/jp107989k</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Methyl and Pentyl Chloride in a Microhydrated Environment and at the Liquid Water-Vapor Interface: A Theoretical Study

  • Original language description

    The solvation properties of methyl and pentyl chloride were studied in microhydrated environment with up to ten explicit water molecules and at the liquid water-vapor interface. Geometry optimizations were performed in the former case using the DFTB, DFTB-D and MP2 levels of theory. Molecular dynamics simulations based on the DFTB and DFTB-D methods were used to study the adsorption process of the alkyl chloride molecules to a water surface. The dynamics simulations show that the methyl chloride molecule is located at the water surface preferentially with the methyl group oriented toward the water surface while for pentyl chloride, owing to the longer non-polar hydrocarbon chain, a parallel alignment at the water surface is found with the hydrocarbon chain pointing slightly to the gas phase.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2011

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Physical Chemistry B

  • ISSN

    1520-6106

  • e-ISSN

  • Volume of the periodical

    115

  • Issue of the periodical within the volume

    8

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    10

  • Pages from-to

    1807-1816

  • UT code for WoS article

    000287636700010

  • EID of the result in the Scopus database