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Complexation of the cesium cation with lithium ionophore VIII: extraction and DFT study

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388963%3A_____%2F13%3A00421967" target="_blank" >RIV/61388963:_____/13:00421967 - isvavai.cz</a>

  • Alternative codes found

    RIV/60460709:41330/13:63623 RIV/60461373:22340/13:43895232

  • Result on the web

    <a href="http://dx.doi.org/10.1007/s10967-013-2686-5" target="_blank" >http://dx.doi.org/10.1007/s10967-013-2686-5</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1007/s10967-013-2686-5" target="_blank" >10.1007/s10967-013-2686-5</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Complexation of the cesium cation with lithium ionophore VIII: extraction and DFT study

  • Original language description

    From extraction experiments and gamma-activity measurements, the extraction constant corresponding to the equilibrium Cs+(aq) + 1 center dot Na (+) (nb) = 1 center dot Cs+(nb) + Na+(aq) taking place in the two-phase water-nitrobenzene system (1 = lithiumionophore VIII; aq = aqueous phase, nb = nitrobenzene phase) was evaluated as log K (ex) (Cs+, 1 center dot Na+) = -0.5 +/- A 0.1. Further, the stability constant of the 1 center dot Cs+ complex in nitrobenzene saturated with water was calculated for atemperature of 25 A degrees C: log beta (nb) (1 center dot Cs+) = 4.8 +/- A 0.2. Finally, by using quantum mechanical DFT calculations, the most probable structure of the cationic complex species 1 center dot Cs+ was derived. In the resulting complex, the "central" cation Cs+ is bound by six bond interactions to the corresponding six oxygen atoms of the parent ligand 1.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CB - Analytical chemistry, separation

  • OECD FORD branch

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2013

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Radioanalytical and Nuclear Chemistry

  • ISSN

    0236-5731

  • e-ISSN

  • Volume of the periodical

    298

  • Issue of the periodical within the volume

    3

  • Country of publishing house

    HU - HUNGARY

  • Number of pages

    4

  • Pages from-to

    2065-2068

  • UT code for WoS article

    000327248400075

  • EID of the result in the Scopus database