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Phosphinate MOFs Formed from Tetratopic Ligands as Proton-Conductive Materials

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388980%3A_____%2F22%3A00557695" target="_blank" >RIV/61388980:_____/22:00557695 - isvavai.cz</a>

  • Alternative codes found

    RIV/68378271:_____/22:00557695 RIV/00216275:25310/22:39918818

  • Result on the web

    <a href="https://doi.org/10.1021/acs.inorgchem.2c00194" target="_blank" >https://doi.org/10.1021/acs.inorgchem.2c00194</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acs.inorgchem.2c00194" target="_blank" >10.1021/acs.inorgchem.2c00194</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Phosphinate MOFs Formed from Tetratopic Ligands as Proton-Conductive Materials

  • Original language description

    Metal-organic frameworks (MOFs) are attracting attention as potential proton conductors. There are two main advantages of MOFs in this application: the possibility of rational design and tuning of the properties and clear conduction pathways given by their crystalline structure. We hereby present two new MOF structures, ICR-10 and ICR-11, based on tetratopic phosphinate ligands. The structures of both MOFs were determined by 3D electron diffraction. They both crystallize in the P3¯ space group and contain arrays of parallel linear pores lined with hydrophilic noncoordinated phosphinate groups. This, together with the adsorbed water molecules, facilitates proton transfer via the Grotthuss mechanism, leading to a proton conductivity of up to 4.26 × 10-4 S cm-1 for ICR-11. The presented study demonstrates the high potential of phosphinate MOFs for the fabrication of proton conductors.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10402 - Inorganic and nuclear chemistry

Result continuities

  • Project

    <a href="/en/project/GA20-04408S" target="_blank" >GA20-04408S: Phosphinic acid based metal-organic frameworks for removal of emerging pollutants and heavy metals</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2022

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Inorganic Chemistry

  • ISSN

    0020-1669

  • e-ISSN

    1520-510X

  • Volume of the periodical

    61

  • Issue of the periodical within the volume

    19

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    7

  • Pages from-to

    7506-7512

  • UT code for WoS article

    000804099400033

  • EID of the result in the Scopus database

    2-s2.0-85130007964