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NMR methods to study effects of additives on phase separation of thermoresponsive polymer

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61389013%3A_____%2F14%3A00428180" target="_blank" >RIV/61389013:_____/14:00428180 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1002/masy.201300130" target="_blank" >http://dx.doi.org/10.1002/masy.201300130</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/masy.201300130" target="_blank" >10.1002/masy.201300130</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    NMR methods to study effects of additives on phase separation of thermoresponsive polymer

  • Original language description

    NMR methods including 1H NMR spectroscopy, 2D NOESY spectroscopy, pulsed-field gradient (PFG) NMR as well as spin-spin relaxation times T2 measurement were employed to study the effects of one surfactant (sodium n-dodecyl sulfate, SDS) and three inorganic salts (NaCl, Na2SO4, Na3PO4) on the phase transition of poly(N-isopropylacrylamide) (PNIPAM) in aqueous solution. The molecular interactions between SDS and PNIPAM during the coil-to-globule transition of PNIPAM have been accurately observed through 2DNOESY spectra and PFG NMR. Through the combination of 1H NMR spectra and T2 measurements, the salts effects have been found not only shift the phase transition of PNIPAM but also lead to difference in the final conformational state of PNIPAM in aqueoussolution after phase transition. Diffusion coefficients of Na+ cations support the idea that the major effect of salts on phase transition of PNIPAM in aqueous solution is produced by anions.

  • Czech name

  • Czech description

Classification

  • Type

    D - Article in proceedings

  • CEP classification

    CD - Macromolecular chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GA13-23392S" target="_blank" >GA13-23392S: Designing and characterization of novel thermosensitive polymer hydrogels</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2014

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Article name in the collection

    Macromolecular Symposia

  • ISBN

  • ISSN

    1022-1360

  • e-ISSN

  • Number of pages

    9

  • Pages from-to

    "Roč. 339"

  • Publisher name

    Wiley

  • Place of publication

    Weinheim

  • Event location

    Prague

  • Event date

    Jul 7, 2013

  • Type of event by nationality

    WRD - Celosvětová akce

  • UT code for WoS article