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Non-isothermal kinetics of cold crystallization in multicomponent PLA/thermoplastic polyurethane/nanofiller system

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61389013%3A_____%2F17%3A00480540" target="_blank" >RIV/61389013:_____/17:00480540 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1007/s10973-017-6417-y" target="_blank" >http://dx.doi.org/10.1007/s10973-017-6417-y</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1007/s10973-017-6417-y" target="_blank" >10.1007/s10973-017-6417-y</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Non-isothermal kinetics of cold crystallization in multicomponent PLA/thermoplastic polyurethane/nanofiller system

  • Original language description

    The effect of platy and tubular nanofillers (NF) in combination with thermoplastic polyurethane (TPU) on cold non-isothermal crystallization (NIC) of poly(lactic acid) (PLA) was studied by differential scanning calorimetry. The data were processed using a recently proposed method of evaluating NIC kinetics. The results indicate that the NF/TPU combination leads to crystallization behaviour of the PLA matrix which is dissimilar from that of the NF-free blend and neat PLA. Addition of organophilized montmorillonite (C30) results in a dual effect on PLA crystallinity—stimulation at lower concentrations and suppression at higher loadings. In the case of halloysite nanotubes (HNT), this effect is practically absent. Crystallinity of injection-moulded samples is significantly increased by cold NIC. This indicates a synergy originating in a complex effect of NF/TPU, e.g. NF-induced changes in morphology and interphase parameters supporting the solid annealing process. TPU partially eliminates negative effect of high NF contents on cold crystallization rate. This effect is more marked in the remelted samples where the rate increases for all NF loadings. This is probably caused by absence of as-prepared crystallites in combination with higher mobility of PLA chains due to presence of TPU. The observed differences between C30 and HNT could be attributed to differences in size, shape, and specific surface. The results indicate that synergistic and antagonistic effects of NF/polymeric modifiers on mechanical and other material parameters are also significantly determined by the effects on crystallization of the matrix.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    20505 - Composites (including laminates, reinforced plastics, cermets, combined natural and synthetic fibre fabrics; filled composites)

Result continuities

  • Project

    <a href="/en/project/GA16-03194S" target="_blank" >GA16-03194S: Effect of modified graphene oxide on performance of multiphase polymer systems</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2017

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Thermal Analysis and Calorimetry

  • ISSN

    1388-6150

  • e-ISSN

  • Volume of the periodical

    130

  • Issue of the periodical within the volume

    2

  • Country of publishing house

    HU - HUNGARY

  • Number of pages

    10

  • Pages from-to

    1043-1052

  • UT code for WoS article

    000413264100046

  • EID of the result in the Scopus database

    2-s2.0-85019055420