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How to force polymer gels to show volume phase transitions

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61389013%3A_____%2F19%3A00502281" target="_blank" >RIV/61389013:_____/19:00502281 - isvavai.cz</a>

  • Result on the web

    <a href="https://pubs.acs.org/doi/10.1021/acsmacrolett.8b00987" target="_blank" >https://pubs.acs.org/doi/10.1021/acsmacrolett.8b00987</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acsmacrolett.8b00987" target="_blank" >10.1021/acsmacrolett.8b00987</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    How to force polymer gels to show volume phase transitions

  • Original language description

    Relatively few polymer gels are known to show volume phase transition where the gels undergo an abrupt change in the degree of swelling by passing through a three-phase equilibrium. Characteristic for such transition is the existence of van der Waals (vdW) loop on the dependence of solvent chemical potential versus polymer concentration. For the χ-induced transition, the existence of vdW loop is determined by the concentration dependence of the interaction function. It is shown that expansive mechanical strains can assist in development of the vdW loop. Systems characterized by continuous change of the degree of swelling transform upon such strain into ones where the degree of swelling changes much and abruptly. Also, expansive modes of strain can make the transition wider and more robust in gels where transition is already observed under free swelling condition. The possibility to induce the volume phase transition by external stresses can be utilized for finding other stimuli sensitive gels, strengthening of gel response, and in modeling of properties of gel constructs by Finite Element Method.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10404 - Polymer science

Result continuities

  • Project

    <a href="/en/project/GA17-08531S" target="_blank" >GA17-08531S: Computational design of hydrogel cell scaffolds.</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2019

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    ACS Macro Letters

  • ISSN

    2161-1653

  • e-ISSN

  • Volume of the periodical

    8

  • Issue of the periodical within the volume

    3

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    7

  • Pages from-to

    272-278

  • UT code for WoS article

    000462098200009

  • EID of the result in the Scopus database

    2-s2.0-85063133256