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Spectroscopic investigations of high-energy-density plasma transformations in a simulated early reducing atmosphere containing methane, nitrogen and water

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61389021%3A_____%2F16%3A00486366" target="_blank" >RIV/61389021:_____/16:00486366 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1039/c6cp05025e" target="_blank" >http://dx.doi.org/10.1039/c6cp05025e</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1039/c6cp05025e" target="_blank" >10.1039/c6cp05025e</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Spectroscopic investigations of high-energy-density plasma transformations in a simulated early reducing atmosphere containing methane, nitrogen and water

  • Original language description

    Large-scale plasma was created in gas mixtures containing methane using high-power laser-induced dielectric breakdown (LIDB). The composition of the mixtures corresponded to a cometary and/or meteoritic impact into the early atmosphere of either Titan or Earth. A multiple-centimeter-sized fireball was created by focusing a single 100 J, 450 ps near-infrared laser pulse into the center of a 15 L gas cell. The excited reaction intermediates formed during the various stages of the LIDB plasma chemical evolution were investigated using optical emission spectroscopy (OES) with temporal resolution. The chemical consequences of laser-produced plasma generation in a CH4-N2-H2O mixture were investigated using high resolution Fourier-transform infrared absorption spectroscopy (FTIR) and gas selected ion flow tube spectrometry (SIFT). Several simple inorganic and organic compounds were identified in the reaction mixture exposed to ten laser sparks. Deuterated water (D2O) in a gas mixture was used to separate several of the produced isotopomers of acetylene, which were then quantified using the FTIR technique.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10305 - Fluids and plasma physics (including surface physics)

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2016

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Physical Chemistry Chemical Physics

  • ISSN

    1463-9076

  • e-ISSN

  • Volume of the periodical

    18

  • Issue of the periodical within the volume

    39

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    9

  • Pages from-to

    27317-27325

  • UT code for WoS article

    000385177200035

  • EID of the result in the Scopus database

    2-s2.0-84991071192