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Metatitanic Acid Pseudomorphs after Titanyl Sulfates: Nanostructured Sorbents and Precursors for Crystalline Titania with Desired Particle Size and Shape

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61988987%3A17310%2F17%3AA1801T5H" target="_blank" >RIV/61988987:17310/17:A1801T5H - isvavai.cz</a>

  • Alternative codes found

    RIV/68378271:_____/17:00480285 RIV/61388980:_____/17:00480285 RIV/46356088:_____/17:N0000035

  • Result on the web

    <a href="http://dx.doi.org/10.1021/acs.cgd.7b01349" target="_blank" >http://dx.doi.org/10.1021/acs.cgd.7b01349</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acs.cgd.7b01349" target="_blank" >10.1021/acs.cgd.7b01349</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Metatitanic Acid Pseudomorphs after Titanyl Sulfates: Nanostructured Sorbents and Precursors for Crystalline Titania with Desired Particle Size and Shape

  • Original language description

    A new preparation method for the synthesis of TiO2 microrods in aqueous media starting with solid hydrated titanyl sulfate crystals with defined morphology is presented. The method is based on the extraction of sulfate ions from the crystals and their replacement with hydroxyl groups in aqueous ammonia solution leaving the Ti-O framework intact. The particle size and morphology of the starting hydrated titanyl sulfate is closely preserved in the pseudomorphs of amorphous metatitanic acid including such details like the layered structure of the original hydrated titanyl sulfate crystals. When annealed up to 1200 degrees C, the rod-like morphology of particles is retained, while the phase composition changes to anatase/rutile. The rod -like particles of metatitanic acid possess excellent sorption properties toward radionuclides. The mechanism of pseudomorph formation is discussed based on the structures of the precursors, including the hitherto unknown structure of titanyl sulfate dihydrate determined by electron diffraction tomography.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10402 - Inorganic and nuclear chemistry

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    V - Vyzkumna aktivita podporovana z jinych verejnych zdroju

Others

  • Publication year

    2017

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    CRYST GROWTH DES

  • ISSN

    1528-7483

  • e-ISSN

    1528-7505

  • Volume of the periodical

    17

  • Issue of the periodical within the volume

    12

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    8

  • Pages from-to

    6762-6769

  • UT code for WoS article

    000417669900069

  • EID of the result in the Scopus database