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Single-Atom (Iron-Based) Catalysts: Synthesis and Applications

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61989100%3A27640%2F21%3A10248976" target="_blank" >RIV/61989100:27640/21:10248976 - isvavai.cz</a>

  • Alternative codes found

    RIV/61989592:15640/21:73611247

  • Result on the web

    <a href="https://pubs.acs.org/doi/pdf/10.1021/acs.chemrev.1c00158" target="_blank" >https://pubs.acs.org/doi/pdf/10.1021/acs.chemrev.1c00158</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acs.chemrev.1c00158" target="_blank" >10.1021/acs.chemrev.1c00158</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Single-Atom (Iron-Based) Catalysts: Synthesis and Applications

  • Original language description

    Supported single-metal atom catalysts (SACs) are constituted of isolated active metal centers, which are heterogenized on inert supports such as graphene, porous carbon, and metal oxides. Their thermal stability, electronic properties, and catalytic activities can be controlled via interactions between the single-metal atom center and neighboring heteroatoms such as nitrogen, oxygen, and sulfur. Due to the atomic dispersion of the active catalytic centers, the amount of metal required for catalysis can be decreased, thus offering new possibilities to control the selectivity of a given transformation as well as to improve catalyst turnover frequencies and turnover numbers. This review aims to comprehensively summarize the synthesis of Fe-SACs with a focus on anchoring single atoms (SA) on carbon/graphene supports. The characterization of these advanced materials using various spectroscopic techniques and their applications in diverse research areas are described. When applicable, mechanistic investigations conducted to understand the specific behavior of Fe-SACs-based catalysts are highlighted, including the use of theoretical models.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10400 - Chemical sciences

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2021

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Chemical Reviews

  • ISSN

    0009-2665

  • e-ISSN

  • Volume of the periodical

    121

  • Issue of the periodical within the volume

    21

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    78

  • Pages from-to

    13620-13697

  • UT code for WoS article

    000718326200010

  • EID of the result in the Scopus database

    2-s2.0-85118274935