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Role of the Cu content and Ce activating effect on catalytic performance of Cu-Mg-Al and Ce/Cu-Mg-Al oxides in ammonia selective catalytic oxidation

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61989100%3A27710%2F22%3A10248130" target="_blank" >RIV/61989100:27710/22:10248130 - isvavai.cz</a>

  • Alternative codes found

    RIV/61989100:27360/22:10248130

  • Result on the web

    <a href="https://www.webofscience.com/wos/woscc/full-record/WOS:000728392000004" target="_blank" >https://www.webofscience.com/wos/woscc/full-record/WOS:000728392000004</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.apsusc.2021.151540" target="_blank" >10.1016/j.apsusc.2021.151540</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Role of the Cu content and Ce activating effect on catalytic performance of Cu-Mg-Al and Ce/Cu-Mg-Al oxides in ammonia selective catalytic oxidation

  • Original language description

    Copper-containing mixed metal oxides were studied as catalysts for selective catalytic oxidation of ammonia. The performed research shows a high correlation between Cu amount and catalyst efficiency, especially dinitrogen selectivity. Copper species, mainly in the form of highly dispersed CuO oxides, were found to be responsible for high N2 selectivity, which decreased with increasing Cu loading and the formation of CuO bulk-like species. The addition of cerium seemed to have an effect on material&apos;s catalytic activity and N2 selectivity. The increase in selectivity towards N2 of Ce-impregnated materials was attributed to the formation of copper-cerium redox couples on the material&apos;s surface. The catalytic tests performed under different NH3/O2 molar ratios revealed that the developed materials exhibit high catalytic activity in a wide range of ammonia concentrations and oxygen contents. (C) 2021 Elsevier B.V.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>ost</sub> - Miscellaneous article in a specialist periodical

  • CEP classification

  • OECD FORD branch

    10402 - Inorganic and nuclear chemistry

Result continuities

  • Project

    <a href="/en/project/EF17_049%2F0008419" target="_blank" >EF17_049/0008419: Support of cross-sectoral cooperation in the field of environmental pollutants reduction and waste recovery</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2022

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Applied Surface Science

  • ISSN

    0169-4332

  • e-ISSN

  • Volume of the periodical

    573

  • Issue of the periodical within the volume

    573 (2022) 151540

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    15

  • Pages from-to

  • UT code for WoS article

  • EID of the result in the Scopus database

    2-s2.0-85117409812