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Stereoselective Synthesis of Benzo[e][1,4]oxazino[4,3-a][1,4]diazepine-6,12-diones with Two Diversity Positions

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61989592%3A15110%2F17%3A73584418" target="_blank" >RIV/61989592:15110/17:73584418 - isvavai.cz</a>

  • Alternative codes found

    RIV/61989592:15310/17:73584418

  • Result on the web

    <a href="http://pubs.acs.org/doi/ipdf/10.1021/acscombsci.7b00134" target="_blank" >http://pubs.acs.org/doi/ipdf/10.1021/acscombsci.7b00134</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acscombsci.7b00134" target="_blank" >10.1021/acscombsci.7b00134</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Stereoselective Synthesis of Benzo[e][1,4]oxazino[4,3-a][1,4]diazepine-6,12-diones with Two Diversity Positions

  • Original language description

    Herein, we report a stereoselective formation of tetrahydro-6H-benzo[e][1,4]oxazino[4,3-a][1,4]diazepine-6,12(11H)-diones. Their preparation consisted in solid-phase synthesis of linear intermediates starting from polymer-supported Ser(tBu)-OH. Using various 2-nitrobenzoic acids and bromoketones, the key intermediates were obtained in five steps and subjected to trifluoroacetic acid-mediated cleavage from the resin followed by stereoselective reduction with triethylsilane. Subsequent catalytic hydrogenation of the nitro group and cyclization yielded the target compounds with full retention of the C12a stereocenter configuration.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10401 - Organic chemistry

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)<br>S - Specificky vyzkum na vysokych skolach

Others

  • Publication year

    2017

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    ACS Combinatorial Science

  • ISSN

    2156-8952

  • e-ISSN

  • Volume of the periodical

    19

  • Issue of the periodical within the volume

    12

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    5

  • Pages from-to

    770-774

  • UT code for WoS article

    000418109500006

  • EID of the result in the Scopus database