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Pd modified prussian blue frameworks: Multiple electron transfer pathways for improving catalytic activity toward hydrogenation of nitroaromatics

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61989592%3A15310%2F20%3A73601967" target="_blank" >RIV/61989592:15310/20:73601967 - isvavai.cz</a>

  • Result on the web

    <a href="https://www.sciencedirect.com/science/article/pii/S2468823120302261" target="_blank" >https://www.sciencedirect.com/science/article/pii/S2468823120302261</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.mcat.2020.110967" target="_blank" >10.1016/j.mcat.2020.110967</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Pd modified prussian blue frameworks: Multiple electron transfer pathways for improving catalytic activity toward hydrogenation of nitroaromatics

  • Original language description

    Prussian blue analogs (PBAs) exhibit potential as low-cost and eco-friendly nanocatalysts that can be fabricated with ease. However, the PBA framework structure suffers from poor electronic conductivity, which limits the catalytic efficiency for this class of materials. Noble metals represent an alternative class of materials that display inherent catalytic activity but suffer from aggregation, ultimately reducing the amount of accessible catalytic sites. Herein, we demonstrate a combinatory approach that circumvents the known disadvantages with these classes of catalytic materials in which PBA-supported nanocatalysts were synthesized. These composite materials exhibit excellent catalytic activity for the reduction of nitroaromatics to aminoaromatics while displaying longterm cycling stability, which is attributed to the availability of multiple electron transfer pathways. Overall, this work opens the study on the assembly of PBA-supported heterogeneous nanocatalysts and potentially paves the way toward future applications.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

  • Continuities

    N - Vyzkumna aktivita podporovana z neverejnych zdroju

Others

  • Publication year

    2020

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Molecular Catalysis

  • ISSN

    2468-8231

  • e-ISSN

  • Volume of the periodical

    492

  • Issue of the periodical within the volume

    AUG

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    9

  • Pages from-to

    "110967-1"-"110967-9"

  • UT code for WoS article

    000549100200009

  • EID of the result in the Scopus database

    2-s2.0-85085374212