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Reaction of Tertiary 2-Chloroketones with Cyanide Ions: Application to 3-Chloroquinolinediones

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F62690094%3A18470%2F21%3A50018879" target="_blank" >RIV/62690094:18470/21:50018879 - isvavai.cz</a>

  • Alternative codes found

    RIV/70883521:28110/21:63536898

  • Result on the web

    <a href="https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/open.202100024" target="_blank" >https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/open.202100024</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/open.202100024" target="_blank" >10.1002/open.202100024</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Reaction of Tertiary 2-Chloroketones with Cyanide Ions: Application to 3-Chloroquinolinediones

  • Original language description

    3-Chloroquinoline-2,4-diones react with cyanide ions in dimethyl formamide to give 3-cyanoquinoline-2,4-diones in small yields due to the strong hindrance of the substituent at the C-3 atom. Good yields can be achieved if the substituent at this position is the methyl group. In the methanol solution, the reaction proceeds by an addition mechanism to form 2-oxo-1a,2,3,7b-tetrahydrooxireno[2,3-c]quinoline-7b-carbonitriles, from which 4-hydroxy-3-methoxy-2-oxo-1,2,3,4-tetrahydroquinoline-4-carbonitriles are subsequently formed by opening of the epoxide ring with methanol. Some minor products of these reactions have also been isolated. The H-1, C-13 and N-15 NMR spectra of the prepared compounds were measured, and all resonances were assigned using appropriate two-dimensional spectra.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10402 - Inorganic and nuclear chemistry

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2021

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    CHEMISTRYOPEN

  • ISSN

    2191-1363

  • e-ISSN

  • Volume of the periodical

    10

  • Issue of the periodical within the volume

    6

  • Country of publishing house

    DE - GERMANY

  • Number of pages

    8

  • Pages from-to

    645-652

  • UT code for WoS article

    000674281000009

  • EID of the result in the Scopus database

    2-s2.0-85108187518