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Perfect Composition Depth Profiling of Ionic Liquid Surfaces Using High-Resolution RBS/ERDA.

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F67985858%3A_____%2F16%3A00463598" target="_blank" >RIV/67985858:_____/16:00463598 - isvavai.cz</a>

  • Alternative codes found

    RIV/44555601:13440/16:43887805

  • Result on the web

    <a href="http://dx.doi.org/10.2116/analsci.32.1089" target="_blank" >http://dx.doi.org/10.2116/analsci.32.1089</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.2116/analsci.32.1089" target="_blank" >10.2116/analsci.32.1089</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Perfect Composition Depth Profiling of Ionic Liquid Surfaces Using High-Resolution RBS/ERDA.

  • Original language description

    In order to reveal the surface structures of large molecular ionic liquids (ILs), the near-surface elemental depth distributions of 1-alkyl 3-methylimidazolium bis(trifluoromethanesulfonyl)imide n([CnC1Im][Tf2N], n = 2, 6, 10) were studied using high-resolution Rutherford backscattering spectroscopy (HRBS) in combination with high-resolution elastic recoil detection analysis (HR-ERDA). nThe elemental depth profiles of all constituent elements, including hydrogen, were derived from HR-ERDA/HRBS measurements, so that the profiles would reproduce both HR-ERDA and HRBS nspectra simultaneously. The derived elemental depth profiles agree with state-of-the-art molecular dynamics simulations, indicating the feasibility of this method. A controversy concerning the preferential orientation of [C2C1Im] at the surface has been resolved by this new combination analysis; namely, the [C2C1Im] cation has a preferential orientation with the ethyl chain pointing to wards the vacuum in the topmost molecular layer.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GA16-12291S" target="_blank" >GA16-12291S: Hierarchical approach to the study of solid-fluid equilibria in complex system: theory, simulation and experiment</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2016

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Analytical Sciences

  • ISSN

    0910-6340

  • e-ISSN

  • Volume of the periodical

    32

  • Issue of the periodical within the volume

    10

  • Country of publishing house

    JP - JAPAN

  • Number of pages

    6

  • Pages from-to

    1089-1094

  • UT code for WoS article

    000386423300010

  • EID of the result in the Scopus database

    2-s2.0-84992521789