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Influence of NaI Additions on the Electrical, Dielectric, and Transport Properties in the GeS2-Ga2S3-NaI Glass System

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F67985891%3A_____%2F19%3A00517260" target="_blank" >RIV/67985891:_____/19:00517260 - isvavai.cz</a>

  • Alternative codes found

    RIV/60461373:22310/19:43919125

  • Result on the web

    <a href="https://link.springer.com/article/10.1134%2FS1023193519060053" target="_blank" >https://link.springer.com/article/10.1134%2FS1023193519060053</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1134/S1023193519060053" target="_blank" >10.1134/S1023193519060053</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Influence of NaI Additions on the Electrical, Dielectric, and Transport Properties in the GeS2-Ga2S3-NaI Glass System

  • Original language description

    The vitreous system GeS2-Ga2S3 can incorporate a large amount of alkali salts, for example NaI, and such materials have a potential to be used as solid electrolytes for all-solid-state batteries. The present work focuses on the effects of NaI addition in the (GeS2)(x)(Ga2S3)(100 -x) glass matrix, where x = 65, 72, 80, and 88. AC and DC electrical and dielectric properties were measured in the temperature range from 20 up to 200 degrees C and in the frequency range 1 Hz-100 kHz, in air, at different temperatures by steps of 1 degrees C. The values of electrical conductivity significantly increase with increasing of NaI content. The DC conductivity values 2.5 x 10(-4) S m(-1) at room temperature were detected for glasses with 25 and 30 mol % of NaI in (GeS2)(72)(Ga2S3)(28) and with 30 mol % NaI in (GeS2)(65)(Ga2S3)(35) matrices. Samples with NaI concentration higher than 20 mol % show a poor stability against moisture. In order to improve their stability the glass composition was modified by addition of 2.5 mol % P2S5 in the system. The activation energy values slightly decrease with NaI content. The GeS2/Ga2S3 ratio and P2S5 addition to the glass matrix have low effect on transport properties. The DC conductivity, electrical relaxation, and depolarization mechanisms are similar. Electrical charge transfer is connected with hopping of Na+ ions or reorientation of dipoles containing theseions.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    20504 - Ceramics

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2019

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Russian Journal of Electrochemistry

  • ISSN

    1023-1935

  • e-ISSN

  • Volume of the periodical

    55

  • Issue of the periodical within the volume

    6

  • Country of publishing house

    RU - RUSSIAN FEDERATION

  • Number of pages

    9

  • Pages from-to

    501-509

  • UT code for WoS article

    000476524300004

  • EID of the result in the Scopus database

    2-s2.0-85069156174