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Re-Modelling of Laves Phases in the Cr-Nb and Cr-Ta Systems Using First-Principles Results

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68081723%3A_____%2F09%3A00325891" target="_blank" >RIV/68081723:_____/09:00325891 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    Re-Modelling of Laves Phases in the Cr-Nb and Cr-Ta Systems Using First-Principles Results

  • Original language description

    Total energies of Laves phases Cr2X, CrX2, CrCr2 and XX2 (X=Nb,Ta) in all three structural forms C14, C15 and C36 have been calculated ab initio by pseudopotential VASP code with a complete relaxation of structural parameters. The calculated values wereused in a two sublattice model for re modelling of Gibbs energies of Laves phases and subsequently for calculation of phase diagrams of Cr Nb and Cr Ta systems by CALPHAD method. It turns out that application of ab initio calculated values of total energy of hypothetical ?end members in a two sublattice model substantially simplifies the modelling and lowers the number of necessary parameters. Comparison of phase diagrams obtained by a model using first principles results with previous empirical approach as well as relative stability of Cr2X polytypes is presented.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    BM - Solid-state physics and magnetism

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GA106%2F07%2F1078" target="_blank" >GA106/07/1078: Theoretical and experimental investigations of thermodynamic properties in transition metal based intermetallic phases</a><br>

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2009

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Calphad - Computer Coupling of Phase Diagrams and Thermochemistry

  • ISSN

    0364-5916

  • e-ISSN

  • Volume of the periodical

    33

  • Issue of the periodical within the volume

    1

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    8

  • Pages from-to

  • UT code for WoS article

    000265006900023

  • EID of the result in the Scopus database