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Decomposition of the single-phase high-entropy alloy CrMnFeCoNi after prolonged anneals at intermediate temperatures

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68081723%3A_____%2F16%3A00464779" target="_blank" >RIV/68081723:_____/16:00464779 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1016/j.actamat.2016.04.005" target="_blank" >http://dx.doi.org/10.1016/j.actamat.2016.04.005</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.actamat.2016.04.005" target="_blank" >10.1016/j.actamat.2016.04.005</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Decomposition of the single-phase high-entropy alloy CrMnFeCoNi after prolonged anneals at intermediate temperatures

  • Original language description

    Among the vast number of multi-principal-element alloys that are referred to as high-entropy alloys (HEAs) in the literature, only a limited number solidify as single-phase solid solutions. The equiatomic HEA, CrMnFeCoNi, is a face-centered cubic (FCC) prototype of this class and has attracted much attention recently because of its interesting mechanical properties. Here we evaluate its phase stability after very long anneals of 500 days at 500-900 degrees C during which it is reasonable to expect thermodynamic equilibrium to have been established. Microstructural analyses were performed using complementary analysis techniques including scanning and transmission electron microscopy (SEM/TEM/STEM), energy dispersive X-ray (EDX) spectroscopy, selected area electron diffraction (SAD), and atom probe tomography (APT). We show that the alloy is a single-phase solid solution after homogenization for 2 days at 1200 degrees C and remains in this state after a subsequent anneal at 900 degrees C for 500 days. However, it is unstable and forms second-phase precipitates at 700 and 500 degrees C. A Cr-rich sigma phase 'forms at 700 degrees C, whereas three different phases (L1(0)-NiMn, B2-FeCo and a Cr-rich body-centered cubic, BCC, phase) precipitate at 500 degrees C. These precipitates are located mostly at grain boundaries, but also form at intragranular inclusions/pores, indicative of heterogeneous nucleation. Since there is limited entropic stabilization of the solid solution state even in the extensively investigated CrMnFeCoNi alloy, the stability of other HEAs currently thought to be solid solutions should be carefully evaluated, especially if they are being considered for applications in vulnerable temperature ranges.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    JG - Metallurgy, metal materials

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GA14-22834S" target="_blank" >GA14-22834S: Phase Stability and Plasticity in Medium-to-High-Entropy Alloys</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2016

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Acta Materialia

  • ISSN

    1359-6454

  • e-ISSN

  • Volume of the periodical

    112

  • Issue of the periodical within the volume

    JUN

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    13

  • Pages from-to

    40-52

  • UT code for WoS article

    000377326400004

  • EID of the result in the Scopus database

    2-s2.0-84963615057