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Superior catalytic properties in aerobic oxidation of olefins over Au nanoparticles on pyrrolidone-modified SBA-15

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68378271%3A_____%2F11%3A00372243" target="_blank" >RIV/68378271:_____/11:00372243 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1016/j.jcat.2011.03.029" target="_blank" >http://dx.doi.org/10.1016/j.jcat.2011.03.029</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.jcat.2011.03.029" target="_blank" >10.1016/j.jcat.2011.03.029</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Superior catalytic properties in aerobic oxidation of olefins over Au nanoparticles on pyrrolidone-modified SBA-15

  • Original language description

    Au nanoparticles highly dispersed in the mesopores of (s)-(?)-2-pyrrolidinone-5-carboxylic acid (Py)-modified SBA-15 (Au/SBA-15-Py) was investigated by using a series of modern techniques 13C NMR and IR spectroscopies XRD, XPS and TEM. Au/SBA-15-Py catalysts always exhibit superior catalytic properties in the oxidation of cyclohexene and styrene by molecular oxygen at atmospheric pressure, compared with the pyrrolidone-free SBA-15 supported Au catalyst (Au/SBA-15-N). This phenomenon is reasonably related to the interaction between Au nanoparticles with Py species, which is consistent with results analyzed from our density-functional theory (DFT) calculations.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    BM - Solid-state physics and magnetism

  • OECD FORD branch

Result continuities

  • Project

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2011

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Catalysis

  • ISSN

    0021-9517

  • e-ISSN

  • Volume of the periodical

    281

  • Issue of the periodical within the volume

    1

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    10

  • Pages from-to

    30-39

  • UT code for WoS article

    000292488600004

  • EID of the result in the Scopus database