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Influence of Ni impurities on the thermoelectric properties of Ca-partially filled skutterudites CaxCo4Sb12.

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68378271%3A_____%2F12%3A00389332" target="_blank" >RIV/68378271:_____/12:00389332 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1063/1.4768439" target="_blank" >http://dx.doi.org/10.1063/1.4768439</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1063/1.4768439" target="_blank" >10.1063/1.4768439</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Influence of Ni impurities on the thermoelectric properties of Ca-partially filled skutterudites CaxCo4Sb12.

  • Original language description

    Polycrystalline samples of the skutterudite compounds CaxCo4Sb12 were synthesized and investigated by means of electrical resistivity, thermal conductivity, and thermopower in the 300?800K temperature range. Additional Hall effect measurements were performed between 2 and 300 K. Both Ni-free and Ni-containing Co powders were used as starting materials to elucidate the impact of Ni impurities at the ppm level on the thermoelectric properties. The presence of minute amounts of Ni atoms in the crystal structure leads to enhanced thermopower values with respect to the Ni-free samples, likely associated with the development of additional electron pockets near the Fermi level.Ni impurities, thus, play a significant role on the transport properties and lead to a spectacular increase in the dimensionless thermoelectric figure of merit ZT of up to 150% at 800 K.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    BM - Solid-state physics and magnetism

  • OECD FORD branch

Result continuities

  • Project

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2012

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Applied Physics Letters

  • ISSN

    0003-6951

  • e-ISSN

  • Volume of the periodical

    101

  • Issue of the periodical within the volume

    22

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    4

  • Pages from-to

    "222105-1"-"222105-4"

  • UT code for WoS article

    000311967000040

  • EID of the result in the Scopus database