Resonant and non-resonant components of the rate of a population transfer in hybrid donor-acceptor systems

Result code in IS VaVaI

<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68378271%3A_____%2F13%3A00421780" target="_blank" >RIV/68378271:_____/13:00421780 - isvavai.cz</a>

Alternative codes found

RIV/61389013:_____/13:00421780

Result on the web

<a href="http://dx.doi.org/10.1166/asem.2013.1337" target="_blank" >http://dx.doi.org/10.1166/asem.2013.1337</a>

DOI - Digital Object Identifier

<a href="http://dx.doi.org/10.1166/asem.2013.1337" target="_blank" >10.1166/asem.2013.1337</a>

Result language

angličtina

Original language name

Resonant and non-resonant components of the rate of a population transfer in hybrid donor-acceptor systems

Original language description

We have studied the charge (or energy) transfer in a two-level hybrid inorganic?organic donor?acceptor system interacting with a vibrational mode embedded in the heat bath. We have shown that the donor population simultaneously decays in time and oscillates with two components corresponding to vibronic transitions 0?0 and 0?1. We have shown that the 0?0 transition decays with longer life-time than the 0?1 component and therefore controls the life-time of the charge (energy) transfer to the acceptor state. We have proved that the rate of the population transfer consists of (I) the non-resonant part given by the Duschinsky coupling in the acceptor state and (II) the resonant part that is additionally controlled by the Huang-Rhys factor of the acceptor state. The resonance appears for integer values of the ratio of energy difference between the donor and the acceptor and the vibrational energy.

Czech name

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Czech description

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Type

J_x - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

CEP classification

BM - Solid-state physics and magnetism

OECD FORD branch

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Project

Result was created during the realization of more than one project. More information in the Projects tab.

Continuities

I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Publication year

2013

Confidentiality

S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Name of the periodical

Advanced Science, Engineering and Medicine

ISSN

2164-6627

e-ISSN

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Volume of the periodical

5

Issue of the periodical within the volume

6

Country of publishing house

US - UNITED STATES

Number of pages

4

Pages from-to

565-568

UT code for WoS article

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EID of the result in the Scopus database

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