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Photocurrent spectroscopy of perovskite layers and solar cells: a sensitive probe of material degradation

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68378271%3A_____%2F17%3A00486914" target="_blank" >RIV/68378271:_____/17:00486914 - isvavai.cz</a>

  • Alternative codes found

    RIV/68407700:21230/17:00308765

  • Result on the web

    <a href="http://dx.doi.org/10.1021/acs.jpclett.6b02854" target="_blank" >http://dx.doi.org/10.1021/acs.jpclett.6b02854</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acs.jpclett.6b02854" target="_blank" >10.1021/acs.jpclett.6b02854</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Photocurrent spectroscopy of perovskite layers and solar cells: a sensitive probe of material degradation

  • Original language description

    Optical absorptance spectroscopy of polycrystalline CH3NH3PbI3 films usually indicates the presence of a PbI2 phase, either as a preparation residue or due to film degradation, but gives no insight on how this may affect electrical properties. Here, we apply photocurrent spectroscopy to both perovskite solar cells and coplanar-contacted layers at various stages of degradation. In both cases, we find that the presence of a PbI2 phase restricts charge-carrier transport, suggesting that PbI2 encapsulates CH3NH3PbI3 grains. We also find that PbI2 injects holes into the CH3NH3PbI3 grains, increasing the apparent photosensitivity of PbI2.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10302 - Condensed matter physics (including formerly solid state physics, supercond.)

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2017

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Physical Chemistry Letters

  • ISSN

    1948-7185

  • e-ISSN

  • Volume of the periodical

    8

  • Issue of the periodical within the volume

    4

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    6

  • Pages from-to

    838-843

  • UT code for WoS article

    000394484100021

  • EID of the result in the Scopus database

    2-s2.0-85013082923