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Autocatalytic surface explosion chemistry of 2D metal-organic frameworks

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68378271%3A_____%2F21%3A00549996" target="_blank" >RIV/68378271:_____/21:00549996 - isvavai.cz</a>

  • Result on the web

    <a href="https://doi.org/10.1021/acs.jpcc.1c03809" target="_blank" >https://doi.org/10.1021/acs.jpcc.1c03809</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acs.jpcc.1c03809" target="_blank" >10.1021/acs.jpcc.1c03809</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Autocatalytic surface explosion chemistry of 2D metal-organic frameworks

  • Original language description

    Metal–organic frameworks are a combination of inorganic constituents and organic ligands with a high degree of variability which are, as coordination compounds in homogeneous catalysis, potentially highly selective heterogeneous catalysts. The synthesis and thermal stability of monolayer thin Cu-, Ni-, and Fe-squarate 2D MOFs are studied using X-ray photoelectron spectroscopy, scanning tunneling microscopy, and temperature-programmed reaction spectroscopy on a Cu(100) surface in ultrahigh vacuum. Highly ordered 2D squarate MOFs are obtained by mild annealing of squarate multilayers. Upon annealing at higher temperatures, the Ni- and Fe-squarate layers undergo autocatalytic surface explosion chemistry with carbon monoxide as a desorbing product in a very narrow temperature interval. Despite the different stabilities of Ni- and Fe-based MOFs, mixed {Ni + Fe}-MOFs also decompose in a narrow single temperature interval.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10302 - Condensed matter physics (including formerly solid state physics, supercond.)

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2021

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Physical Chemistry C

  • ISSN

    1932-7447

  • e-ISSN

    1932-7455

  • Volume of the periodical

    125

  • Issue of the periodical within the volume

    24

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    7

  • Pages from-to

    13343-13349

  • UT code for WoS article

    000668350500026

  • EID of the result in the Scopus database

    2-s2.0-85108868805