Terahertz magnetic and lattice excitations in van der Waals ferromagnet VI3
The result's identifiers
Result code in IS VaVaI
<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68378271%3A_____%2F22%3A00564655" target="_blank" >RIV/68378271:_____/22:00564655 - isvavai.cz</a>
Alternative codes found
RIV/00216208:11320/22:10451724 RIV/68407700:21340/22:00361858
Result on the web
<a href="https://doi.org/10.1021/acs.jpclett.2c02944" target="_blank" >https://doi.org/10.1021/acs.jpclett.2c02944</a>
DOI - Digital Object Identifier
<a href="http://dx.doi.org/10.1021/acs.jpclett.2c02944" target="_blank" >10.1021/acs.jpclett.2c02944</a>
Alternative languages
Result language
angličtina
Original language name
Terahertz magnetic and lattice excitations in van der Waals ferromagnet VI3
Original language description
We use the synergy of infrared, terahertz, and Raman spectroscopies with DFT calculations to shed light on the magnetic and lattice properties of VI3. The structural transition at TS1 = 79 K is accompanied by a large splitting of polar phonon modes. Below TS1, strong ferromagnetic fluctuations are observed. The variations of phonon frequencies at 55 K induced by magnetoelastic coupling enhanced by spin−orbit interaction indicate the proximity of long-range ferromagnetic order. Below TC = 50 K, two Raman modes simultaneously appear and show dramatic softening in the narrow interval around the temperature TS2 of the second structural transition associated with the order−order magnetic phase transition. Below TS2, a magnon in the THz range appears in Raman spectra. The THz magnon observed in VI3 indicates the application potential of 2D van der Waals ferromagnets in ultrafast THz spintronics.
Czech name
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Czech description
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Classification
Type
J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database
CEP classification
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OECD FORD branch
10302 - Condensed matter physics (including formerly solid state physics, supercond.)
Result continuities
Project
Result was created during the realization of more than one project. More information in the Projects tab.
Continuities
I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace
Others
Publication year
2022
Confidentiality
S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů
Data specific for result type
Name of the periodical
Journal of Physical Chemistry Letters
ISSN
1948-7185
e-ISSN
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Volume of the periodical
13
Issue of the periodical within the volume
30
Country of publishing house
US - UNITED STATES
Number of pages
10
Pages from-to
11095-11104
UT code for WoS article
000891130800001
EID of the result in the Scopus database
2-s2.0-85143081551