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Silver vapor supersonic jets: expansion dynamics, cluster formation, and film deposition

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68378271%3A_____%2F23%3A00573862" target="_blank" >RIV/68378271:_____/23:00573862 - isvavai.cz</a>

  • Result on the web

    <a href="https://hdl.handle.net/11104/0344221" target="_blank" >https://hdl.handle.net/11104/0344221</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.3390/ma16134876" target="_blank" >10.3390/ma16134876</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Silver vapor supersonic jets: expansion dynamics, cluster formation, and film deposition

  • Original language description

    Supersonic jets of metal vapors with carrier gas are promising for producing nanostructured metal films at relatively low source temperatures and high deposition rates.Effects of the carrier gas on the jet composition and expansion dynamics,as well as on film properties,remain virtually unexplored.In this work,the free-jet expansion of a mixture of silver vapor with helium in a rarefied regime at an initial temperature of 1373 K is investigated through mass spectrometry and direct-simulation Monte Carlo methods.Introducing the carrier gas into the source is found to result in a transition from a collisionless to a collision-dominated expansion regime and dramatic changes in the Ag jet,which becomes denser,faster,and more forward-directed.The changes are shown to be favorable for the formation of small Ag clusters and film deposition.At a fairly high helium flow,silver Ag2 dimers are observed in the jet,both in the experiment and the simulations,with a mole fraction reaching 0.1%.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10306 - Optics (including laser optics and quantum optics)

Result continuities

  • Project

    <a href="/en/project/EF15_003%2F0000445" target="_blank" >EF15_003/0000445: Advanced designing of functional materials: From mono- to BI- And TRI-chromatic excitation with tailored laser pulses</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2023

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Materials

  • ISSN

    1996-1944

  • e-ISSN

    1996-1944

  • Volume of the periodical

    16

  • Issue of the periodical within the volume

    13

  • Country of publishing house

    CH - SWITZERLAND

  • Number of pages

    26

  • Pages from-to

    4876

  • UT code for WoS article

    001028581500001

  • EID of the result in the Scopus database

    2-s2.0-85165083437