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5f-electron localization in uranium binary hydrides: Photoelectron spectroscopy

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68378271%3A_____%2F24%3A00587248" target="_blank" >RIV/68378271:_____/24:00587248 - isvavai.cz</a>

  • Alternative codes found

    RIV/00216208:11320/24:10481798

  • Result on the web

    <a href="https://doi.org/10.1103/PhysRevB.109.075165" target="_blank" >https://doi.org/10.1103/PhysRevB.109.075165</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1103/PhysRevB.109.075165" target="_blank" >10.1103/PhysRevB.109.075165</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    5f-electron localization in uranium binary hydrides: Photoelectron spectroscopy

  • Original language description

    The relation of 5f-electron localization and valence-band x-ray and ultraviolet photoelectron spectra (XPS, UPS) is analyzed on the example of uranium binary hydrides. Confronted with results of density functional theory calculations, it is recognized that electron-electron correlations play an important role. The spectra can be well accounted for by dynamical mean-field theory (DMFT) calculations providing insight into the final state remaining after the photoexcitation event. Details of the spectra reflect the dominant final-state 5f2 multiplets with the main line adjacent to the Fermi level and the first excited line responsible for a shoulder at 0.5 eV binding energy.Calculations with a varied strength of hybridization between 5f and non-f states allow us to visualize how the individual multiplet lines shift in energy.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10302 - Condensed matter physics (including formerly solid state physics, supercond.)

Result continuities

  • Project

    <a href="/en/project/GA21-09766S" target="_blank" >GA21-09766S: Magnetism and electronic structure of actinides tuned by ionicity</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2024

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Physical Review B

  • ISSN

    2469-9950

  • e-ISSN

    2469-9969

  • Volume of the periodical

    109

  • Issue of the periodical within the volume

    7

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    9

  • Pages from-to

    075165

  • UT code for WoS article

    001198654800001

  • EID of the result in the Scopus database

    2-s2.0-85186365311