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Mercury species in formerly contaminated soils and released soil gases

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68407700%3A21340%2F17%3A00340766" target="_blank" >RIV/68407700:21340/17:00340766 - isvavai.cz</a>

  • Alternative codes found

    RIV/61389005:_____/17:00474577 RIV/00216224:14310/17:00094664

  • Result on the web

    <a href="https://doi.org/10.1016/j.scitotenv.2017.01.157" target="_blank" >https://doi.org/10.1016/j.scitotenv.2017.01.157</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.scitotenv.2017.01.157" target="_blank" >10.1016/j.scitotenv.2017.01.157</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Mercury species in formerly contaminated soils and released soil gases

  • Original language description

    Total mercury (T-Hg), elemental mercury (Hg-0), methylmercury (MeHg+), phenylmercury (PhHg+), and gaseous elemental mercury (GEM) species were determined in soils formerly contaminated by different processes from two sites in the Czech Republic. Analytical methods involved atomic absorption spectrometry (AAS) using a single-purpose Advanced Mercury Analyser AMA-254 and radiochemical neutron activation analysis (RNAA) for T-Hg determination, a thermal desorption method was used for Hg-0 determination, gas chromatography coupled with atomic fluorescence spectrometry (GC-AFS) was employed for assay of MeHg+ and PhHg+, while GEM measurement was carried out using a portable Zeeman AAS device Lumex RA-915(+). The first sampling site was in the surroundings of a former PhHgCl-based fungicide processing plant next to Pribram (central Bohemia). Although the use of Hg-based fungicides as seed mordant have been banned, and their production stopped at the end of 1980's, highly elevated Hg contents in soil are still observed in the vicinity of the former plant, reaching T-Hg values >13 mg kg(-1). The second sampling site was an abandoned mining area named Jedova hora Hill near Horovice (central Bohemia), where cinnabar (HgS) was occasionally mined as by-product of Fe ores hematite and siderite. Mining activities have been stopped here in 1857. Very high contents of T-Hg are still found at this site, up to 144 mg kg(-1). In most cases we found a statistically significant correlation between T-Hg and Hg-0 values regardless of the pollution source. On the contrary, insignificant correlation was observed neither between T-Hg and GEM values, nor between GEM and Hg. Concentrations of the investigated organomercury species were above a limit of detection (LOD) only in the most contaminated samples, where their levels were about two to three orders of magnitude lower compared to those of T-Hg. (C) 2017 Elsevier B.V. All rights reserved.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10406 - Analytical chemistry

Result continuities

  • Project

  • Continuities

    V - Vyzkumna aktivita podporovana z jinych verejnych zdroju

Others

  • Publication year

    2017

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    The Science of the Total Environment

  • ISSN

    0048-9697

  • e-ISSN

    1879-1026

  • Volume of the periodical

    584

  • Issue of the periodical within the volume

    Duben

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    8

  • Pages from-to

    1032-1039

  • UT code for WoS article

    000399358500100

  • EID of the result in the Scopus database

    2-s2.0-85028272411