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Photoluminescence Spectra and Unusual Temperature Shift of Zero-Phonon Emission Line of V3+ in SrTiO3

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68407700%3A21340%2F23%3A00373685" target="_blank" >RIV/68407700:21340/23:00373685 - isvavai.cz</a>

  • Result on the web

    <a href="https://doi.org/10.1134/S0030400X23040197" target="_blank" >https://doi.org/10.1134/S0030400X23040197</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1134/S0030400X23040197" target="_blank" >10.1134/S0030400X23040197</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Photoluminescence Spectra and Unusual Temperature Shift of Zero-Phonon Emission Line of V3+ in SrTiO3

  • Original language description

    The paper presents the first observation of photoluminescence spectra of V3+ impurity in SrTiO3. The broad band of the observed emission is located in the near IR region and at low temperatures consists of a pronounced zero-phonon line (ZPL) with a maximum at 1157.1 nm (8642 cm–1) at 77 K and developed vibronic sidebands extending to 1450 nm. The observed ZPL is associated with an intracenter 1T2g -> 3T1g or a closely located 1Eg -> 3T1g emission transition in V3+ (3d2) ions replacing Ti4+ ions. It was found that the temperature shift of zero-phonon line is unusually large and its frequency decreases upon lowering the temperature. The local configuration instability of V3+ ions in the 3T1g ground state caused by soft TO1 temperature-dependent phonon mode present in SrTiO3 is considered as a possible source of the observed unusual temperature shift.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>SC</sub> - Article in a specialist periodical, which is included in the SCOPUS database

  • CEP classification

  • OECD FORD branch

    10306 - Optics (including laser optics and quantum optics)

Result continuities

  • Project

    <a href="/en/project/EF16_019%2F0000778" target="_blank" >EF16_019/0000778: Center for advanced applied science</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2023

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Optics and Spectroscopy

  • ISSN

    0030-400X

  • e-ISSN

    1562-6911

  • Volume of the periodical

    131

  • Issue of the periodical within the volume

    3

  • Country of publishing house

    CH - SWITZERLAND

  • Number of pages

    4

  • Pages from-to

    183-186

  • UT code for WoS article

  • EID of the result in the Scopus database

    2-s2.0-85187793854