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The degradation of poly(1-butene) extrudates subjected to artificial and natural aging

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F70883521%3A28110%2F24%3A63579858" target="_blank" >RIV/70883521:28110/24:63579858 - isvavai.cz</a>

  • Result on the web

    <a href="https://link.springer.com/article/10.1007/s13726-024-01348-z" target="_blank" >https://link.springer.com/article/10.1007/s13726-024-01348-z</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1007/s13726-024-01348-z" target="_blank" >10.1007/s13726-024-01348-z</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    The degradation of poly(1-butene) extrudates subjected to artificial and natural aging

  • Original language description

    In this work, we examined the degradation behavior of isotactic poly(1-butene) (PB-1) under artificial aging and natural weathering conditions. PB-1 samples underwent accelerated aging through UV irradiation and natural weathering. Chemical and structural changes in the degraded samples were characterized using Fourier-transform infrared–attenuated total reflectance (FTIR–ATR) spectroscopy, surface analysis, and wide-angle X-ray scattering (WAXS). The mechanical properties were evaluated via tensile testing. FTIR–ATR analysis revealed the presence of carbonyl groups in the degraded samples, indicating oxidative degradation. Surface observations employing scanning electron microscopy (SEM) revealed the formation of surface cracks in both samples, with differing crack initiation mechanisms. The two aging methods affected the mechanical properties of the samples: artificial aging induced a gradual reduction in both tensile modulus and strength, whereas natural weathering engendered a marginal increment in modulus alongside diminished strength. Additionally, elongation-at-break value witnessed a marked decrease in both sample sets during the preliminary stages of degradation. This work employed accelerated time equivalent, obtained by juxtaposition of the values of carbonyl index during both artificial aging and natural weathering and their interpolation to determine the degradation rate and adequately to correlate the final properties of the aged PB-1. It was observed that surface morphology and mechanical attributes of degraded samples were subject to additional influences such as temperature, humidity, and precipitation during natural weathering. This research work provided significant insights into PB-1 degradation mechanisms and effect of different aging conditions on its performance.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10404 - Polymer science

Result continuities

  • Project

  • Continuities

    S - Specificky vyzkum na vysokych skolach

Others

  • Publication year

    2024

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Iranian Polymer Journal

  • ISSN

    1026-1265

  • e-ISSN

    1735-5265

  • Volume of the periodical

    33

  • Issue of the periodical within the volume

    12

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    11

  • Pages from-to

    1725-1735

  • UT code for WoS article

    001251083900001

  • EID of the result in the Scopus database

    2-s2.0-85196412669