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A tertiary amine in two competitive processes: Reduction of graphene oxide vs. catalysis of atom transfer radical polymerization

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F70883521%3A28610%2F15%3A43873056" target="_blank" >RIV/70883521:28610/15:43873056 - isvavai.cz</a>

  • Result on the web

    <a href="http://pubs.rsc.org/en/content/articlelanding/2014/ra/c4ra12915f/unauth#!divAbstract" target="_blank" >http://pubs.rsc.org/en/content/articlelanding/2014/ra/c4ra12915f/unauth#!divAbstract</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1039/c4ra12915f" target="_blank" >10.1039/c4ra12915f</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    A tertiary amine in two competitive processes: Reduction of graphene oxide vs. catalysis of atom transfer radical polymerization

  • Original language description

    Electrically conductive graphene oxide-polystyrene hybrids (GO-PS) were prepared by reduction of graphene oxide (GO) in one step during covalent modification of graphene oxide surface using surface-initiated atom transfer radical polymerization (SI-ATRP)of styrene. The reduction of the GO surface was proven by Raman spectroscopy, electrical conductivity measurements, thermogravimetric analysis and X-ray photoelectron spectroscopy. Electrical conductivity of the synthesized GO-PS particles increased ineight orders of magnitude, depending on the polymerization period. Detailed studies were performed to determine that the tertiary amine, such as N,N,N',N',N"-pentamethyldiethylenetriamine (PMDETA), used in SI-ATRP as a ligand complexing copper catalyst,was responsible for the GO surface reduction. It was shown that due to participation of PMDETA in reduction of graphene oxide, the ATRP in the presence of GO can proceed only above a certain PMDETA-GO ratio.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CD - Macromolecular chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/ED2.1.00%2F03.0111" target="_blank" >ED2.1.00/03.0111: Centre of Polymer Systems</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2015

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    RSC Advances: an international journal to further the chemical sciences

  • ISSN

    2046-2069

  • e-ISSN

  • Volume of the periodical

    5

  • Issue of the periodical within the volume

    5

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    7

  • Pages from-to

    3370-3376

  • UT code for WoS article

    000346405200029

  • EID of the result in the Scopus database