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ABA and BAB Triblock Copolymers Based on 2-Methyl-2-oxazoline and 2-n-Propyl-2-oxazoline: Synthesis and Thermoresponsive Behavior in Water

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F70883521%3A28610%2F17%3A63516640" target="_blank" >RIV/70883521:28610/17:63516640 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1002/macp.201700031" target="_blank" >http://dx.doi.org/10.1002/macp.201700031</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/macp.201700031" target="_blank" >10.1002/macp.201700031</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    ABA and BAB Triblock Copolymers Based on 2-Methyl-2-oxazoline and 2-n-Propyl-2-oxazoline: Synthesis and Thermoresponsive Behavior in Water

  • Original language description

    Inspired by the well-known amphiphilic block copolymer platform known as Pluronics or poloxamers, a small library of ABA and BAB triblock copolymers comprising hydrophilic 2-methyl-2-oxazoline (A) and thermoresponsive 2-n-propyl-2-oxazoline (B) is synthesized. These novel copolymers exhibit temperature-induced self-assembly in aqueous solution. The formation and size of aggregates depend on the polymer structure, temperature, and concentration. The BAB copolymers tend to agglomerate in water, with the cloud point temperature depending on the length of poly(2-n-propyl-2-oxazoline) chain. On the other hand, ABA copolymers form smaller aggregates with hydrodynamic radius from 25 to 150 nm. The dependence of viscosity and viscoelastic properties on the temperature is also studied. While several Pluronic block copolymers are known to form thermoreversible hydrogels in the concentration range 20–30 wt%, thermogelation is not observed for any of the investigated poly(2-oxazoline)s at the investigated temperature range from 10 to 50 °C. (Figure presented.).

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10404 - Polymer science

Result continuities

  • Project

    <a href="/en/project/LO1504" target="_blank" >LO1504: Centre of Polymer Systems Plus</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2017

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Macromolecular chemistry and Physics

  • ISSN

    1022-1352

  • e-ISSN

  • Volume of the periodical

    218

  • Issue of the periodical within the volume

    13

  • Country of publishing house

    DE - GERMANY

  • Number of pages

    12

  • Pages from-to

  • UT code for WoS article

    000404903000011

  • EID of the result in the Scopus database

    2-s2.0-85018806665