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In situ generation of copper cations and complexation with tebuconazole in a hyphenation of electrochemistry with mass spectrometry

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11310%2F13%3A10144179" target="_blank" >RIV/00216208:11310/13:10144179 - isvavai.cz</a>

  • Alternative codes found

    RIV/61388963:_____/13:00393011 RIV/60460709:41210/13:61987

  • Result on the web

    <a href="http://dx.doi.org/10.1016/j.ijms.2013.01.005" target="_blank" >http://dx.doi.org/10.1016/j.ijms.2013.01.005</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.ijms.2013.01.005" target="_blank" >10.1016/j.ijms.2013.01.005</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    In situ generation of copper cations and complexation with tebuconazole in a hyphenation of electrochemistry with mass spectrometry

  • Original language description

    Tebuconazole (1) belongs to a class of widely utilized plant fungicides, mostly in vineyards. Consequently, traces of this compound are present in plant tissues, wine as well as in soil. The aim of this study was in situ generation of Cu cations and creation of very stable Cu complexes with 1. The proposed method involves a hyphenation of electrochemistry with electrospray ionization mass spectrometry (ESI-MS), based on the high affinity of 1 for dissolved copper cations. We demonstrate that at appropriate potentials (above 500 mV vs. silver reference electrode) Cu cations can be generated in an electrochemical cell, which subsequently form complexes with 1 present in the sample. The resulting complex [Cu(1)](+) as well as its fragment [Cu(1-C4H10)](+)are then detected with online-coupled ESI-MS. This finding is useful for a creation of an analytical method based on the detection of trace amounts of 1 in complex matrices (e.g., soil solution), in which the analyte may be spread among

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CG - Electrochemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GP13-21409P" target="_blank" >GP13-21409P: Interactions of metal and nutrient ions with high priority pesticides in soil and on biomembranes</a><br>

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)<br>S - Specificky vyzkum na vysokych skolach<br>I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2013

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    International Journal of Mass Spectrometry

  • ISSN

    1387-3806

  • e-ISSN

  • Volume of the periodical

    338

  • Issue of the periodical within the volume

    March

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    5

  • Pages from-to

    45-49

  • UT code for WoS article

    000317444600008

  • EID of the result in the Scopus database