Observation of stimulated Raman scattering in polar tetragonal crystals of barium antimony tartrate trihydrate, Ba[Sb-2((+)C4H2O6)(2)].3H2O
Result description
The non-centrosymmetric polar tetragonal (P4(1)) barium antimony tartrate trihydrate, Ba[Sb-2((+)C4H2O6)(2)].3H2O, was found to be an attractive novel semi-organic crystal manifesting numerous chi((2)-) and chi((3)-)nonlinear optical interactions. In particular, with picosecond single- and dual-wavelength pumping SHG and THG via cascaded parametric four-wave processes were observed. High-order Stokes and anti-Stokes lasing related to two SRS-promoting vibration modes of the crystal, with omega(SRS1) approximate to 575 cm(-1) and omega(SRS2) approximate to 2940 cm(-1), takes place. Basing on a spontaneous Raman investigation an assignment of the two SRS-active vibration modes is discussed.
Keywords
barium antimony tartrate trihydrateBa[Sb-2((+)C4H2O6)(2)].3H2O single crystalchi((3))-nonlinear Stokes and anti-Stokes lasingthird harmonic generation (THG)second harmonic generation (SHG)stimulated Raman scattering (SRS)
The result's identifiers
Result code in IS VaVaI
Result on the web
DOI - Digital Object Identifier
Alternative languages
Result language
angličtina
Original language name
Observation of stimulated Raman scattering in polar tetragonal crystals of barium antimony tartrate trihydrate, Ba[Sb-2((+)C4H2O6)(2)].3H2O
Original language description
The non-centrosymmetric polar tetragonal (P4(1)) barium antimony tartrate trihydrate, Ba[Sb-2((+)C4H2O6)(2)].3H2O, was found to be an attractive novel semi-organic crystal manifesting numerous chi((2)-) and chi((3)-)nonlinear optical interactions. In particular, with picosecond single- and dual-wavelength pumping SHG and THG via cascaded parametric four-wave processes were observed. High-order Stokes and anti-Stokes lasing related to two SRS-promoting vibration modes of the crystal, with omega(SRS1) approximate to 575 cm(-1) and omega(SRS2) approximate to 2940 cm(-1), takes place. Basing on a spontaneous Raman investigation an assignment of the two SRS-active vibration modes is discussed.
Czech name
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Czech description
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Classification
Type
Jimp - Article in a specialist periodical, which is included in the Web of Science database
CEP classification
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OECD FORD branch
10306 - Optics (including laser optics and quantum optics)
Result continuities
Project
GA14-05506S: Crystal engineering of novel molecular crystals for non-linear optics
Continuities
P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)
Others
Publication year
2017
Confidentiality
S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů
Data specific for result type
Name of the periodical
Annalen der Physik
ISSN
0003-3804
e-ISSN
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Volume of the periodical
529
Issue of the periodical within the volume
4
Country of publishing house
DE - GERMANY
Number of pages
9
Pages from-to
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UT code for WoS article
000399307700009
EID of the result in the Scopus database
2-s2.0-85011361625
Basic information
Result type
Jimp - Article in a specialist periodical, which is included in the Web of Science database
OECD FORD
Optics (including laser optics and quantum optics)
Year of implementation
2017