Molecular Auger Interferometry
The result's identifiers
Result code in IS VaVaI
<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F19%3A10405654" target="_blank" >RIV/00216208:11320/19:10405654 - isvavai.cz</a>
Result on the web
<a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=En_fKqHH8n" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=En_fKqHH8n</a>
DOI - Digital Object Identifier
<a href="http://dx.doi.org/10.1103/PhysRevLett.122.233001" target="_blank" >10.1103/PhysRevLett.122.233001</a>
Alternative languages
Result language
angličtina
Original language name
Molecular Auger Interferometry
Original language description
We introduce and present a theory of interferometric measurement of a normal Auger decay lifetime in molecules. Molecular Auger interferometry is based on the coherent phase control of Auger dynamics in a two-color (omega/2 omega) laser field. We show that, in contrast to atoms, in oriented molecules of certain point groups the relative omega/2 omega phase modulates the total ionization yield. A simple analytical formula is derived for the extraction of the lifetimes of Auger-active states from a molecular Auger interferogram, circumventing the need in either high-resolution or attosecond spectroscopy. We demonstrate the principle of the interferometric Auger lifetime measurement using inner-valence decay in CH3F.
Czech name
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Czech description
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Classification
Type
J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database
CEP classification
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OECD FORD branch
10301 - Atomic, molecular and chemical physics (physics of atoms and molecules including collision, interaction with radiation, magnetic resonances, Mössbauer effect)
Result continuities
Project
<a href="/en/project/GA17-10866S" target="_blank" >GA17-10866S: Properties of autoionizing states in atoms, molecules and clusters</a><br>
Continuities
P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)
Others
Publication year
2019
Confidentiality
S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů
Data specific for result type
Name of the periodical
Physical Review Letters
ISSN
0031-9007
e-ISSN
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Volume of the periodical
122
Issue of the periodical within the volume
23
Country of publishing house
US - UNITED STATES
Number of pages
6
Pages from-to
233001
UT code for WoS article
000471988300005
EID of the result in the Scopus database
2-s2.0-85067339714