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Sputter-etching treatment of proton-exchange membranes: Completely dry thin-film approach to low-loading catalyst-coated membranes for water electrolysis

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F20%3A10413956" target="_blank" >RIV/00216208:11320/20:10413956 - isvavai.cz</a>

  • Result on the web

    <a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=oR0MWkFrY7" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=oR0MWkFrY7</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.ijhydene.2020.05.245" target="_blank" >10.1016/j.ijhydene.2020.05.245</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Sputter-etching treatment of proton-exchange membranes: Completely dry thin-film approach to low-loading catalyst-coated membranes for water electrolysis

  • Original language description

    Simultaneous plasma etching of a proton-exchange membrane (PEM) and deposition of a cerium oxide layer during reactive magnetron sputtering leads to the formation of a pronounced fiber-like structure on its surface. The level of structural porosity can be adjusted by varying the working pressure during the process. A PEM treated this way can be subsequently coated with a thin layer of iridium, forming an anode-side catalyst-coated membrane (CCM) for applications in water electrolysis. Due to the significantly enlarged surface of the membrane, there is no necessity for any additional, potentially corroding, support nanoparticles to achieve efficient in-cell operation. Moreover, utilizing a rotatory frame-shaped substrate holder and a multitarget deposition apparatus, the sputter-etching process can be used in the preparation of a full anode/cathode thin-film CCM in a single vacuum entry. This structure yields remarkable performance characteristics in an electrolyzer cell, considering its low combined noble metal loading of just 220 mu g cm(-2). Using this completely dry process for CCM manufacturing may facilitate efficient large-scale future production. (C) 2020 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10305 - Fluids and plasma physics (including surface physics)

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2020

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    International Journal of Hydrogen Energy

  • ISSN

    0360-3199

  • e-ISSN

  • Volume of the periodical

    45

  • Issue of the periodical within the volume

    41

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    11

  • Pages from-to

    20776-20786

  • UT code for WoS article

    000558598300006

  • EID of the result in the Scopus database

    2-s2.0-85086934508