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Microcalorimetric and FTIR study of the adsorption of carbon dioxide on alkali-metal exchanged FER zeolites

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216275%3A25310%2F10%3A39881899" target="_blank" >RIV/00216275:25310/10:39881899 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    Microcalorimetric and FTIR study of the adsorption of carbon dioxide on alkali-metal exchanged FER zeolites

  • Original language description

    Adsorption of CO2 on alkali-metal exchanged (Li+, Na+, K+) FER zeolites was investigated by means of microcalorimetry and FTIR spectroscopy. The adsorption enthalpies strongly depend on coverage for all investigated materials and they are also influencedby concentration of Al in the framework. Especially, samples of Na- and K-FER with lower Si/Al ratio (8.6) exhibited substantially larger initial interaction energy than samples with Si/Al 27.5. Differences in zero-coverage adsorption energy of zeoliteswith different cation concentration (Si/Al ratio) are 9 and 7.2 kJ/mol for Na- and K-FER zeolites respectively. This phenomenon is attributed to formation of bridged CO2 adsorption complexes formed between two cations, which are characterized by IR absorption band of ný3 stretching vibration mode at 2370 and 2357 cm-1 for Na- and K-FER respectively.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2010

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Topics in Catalysis

  • ISSN

    1022-5528

  • e-ISSN

  • Volume of the periodical

    53

  • Issue of the periodical within the volume

    19-20

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    12

  • Pages from-to

  • UT code for WoS article

    000283584800009

  • EID of the result in the Scopus database