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How to elucidate and control the redox sequence in vinylbenzoate and vinylpyridine bridged diruthenium complexes

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F10%3A00349519" target="_blank" >RIV/61388955:_____/10:00349519 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    How to elucidate and control the redox sequence in vinylbenzoate and vinylpyridine bridged diruthenium complexes

  • Original language description

    Vinylbenzoate-bridged diruthenium complexes (RHCdouble bond, length as m-dashCH)(CO)(PiPr3)2Ru(?-4-OOCC6H4?CHdouble bond, length as m-dashCH)RuCl(CO)(PiPr3)2 (R = Ph, 3a or CF3, 3b) and vinylpyridine-bridged (?6-p-cymene)Cl2Ru(?-NC5H4-4-CHdouble bond, length as m-dashCH)RuCl(CO)(PiPr3)2 (3c) have been prepared from their monoruthenium precursors and investigated with respect to the sequence of the individual redox steps and electron delocalization in their partially and fully oxidized states. Identification of the primary redox sites rests on the trends in redox potentials and the EPR, IR and Vis/NIR signatures of the oxidized radical cations and is correctly reproduced by quantum chemical investigations.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CG - Electrochemistry

  • OECD FORD branch

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)<br>Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2010

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Dalton Transactions

  • ISSN

    1477-9226

  • e-ISSN

  • Volume of the periodical

    39

  • Issue of the periodical within the volume

    34

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    12

  • Pages from-to

  • UT code for WoS article

    000281109800020

  • EID of the result in the Scopus database