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Acylation of p-xylene over zeolites

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F12%3A00375911" target="_blank" >RIV/61388955:_____/12:00375911 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1016/j.cattod.2011.06.033" target="_blank" >http://dx.doi.org/10.1016/j.cattod.2011.06.033</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.cattod.2011.06.033" target="_blank" >10.1016/j.cattod.2011.06.033</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Acylation of p-xylene over zeolites

  • Original language description

    Zeolites differing in structure and acidity were tested in liquid phase acylation of p-xylene. Hexanoyl chloride, propionic anhydride and isobutyric anhydride were used as acylating agents. The highest conversions of acylating agent were achieved over large pore zeolites USY (66.3%) and Beta (58.2%). It was found that acylation of p-xylene proceeds only over large pore zeolites Beta and USY. Selectivities to monoacylated p-xylene obtained over USY zeolite decreased in the order: propionic anhydride 78.0% > hexanoyl chloride 67.2% > isobutyric anhydride 33.1%. Diacylated product was formed over zeolite USY with all acylating agents tested but only with hexanoyl chloride over zeolite Beta. It was found that the optimum Si/Al ratio of zeolite Beta for p-xylene acylation with propionic anhydride is 25, while for isobutyric anhydride is 19. Conversion of isobutyric anhydride decreased with increasing isobutyric anhydride concentration and increased with increasing amount of catalyst.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2012

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Catalysis Today

  • ISSN

    0920-5861

  • e-ISSN

  • Volume of the periodical

    179

  • Issue of the periodical within the volume

    1

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    7

  • Pages from-to

    78-84

  • UT code for WoS article

    000298404600010

  • EID of the result in the Scopus database