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Metathesis of cardanol over Ru catalysts supported on mesoporousmolecular sieve SBA-15

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F14%3A00427729" target="_blank" >RIV/61388955:_____/14:00427729 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1016/j.apcata.2014.03.036" target="_blank" >http://dx.doi.org/10.1016/j.apcata.2014.03.036</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.apcata.2014.03.036" target="_blank" >10.1016/j.apcata.2014.03.036</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Metathesis of cardanol over Ru catalysts supported on mesoporousmolecular sieve SBA-15

  • Original language description

    tThe Hoveyda?Grubbs type Zhan catalysts (ZC) and Grubbs second generation catalyst (GII) were immo-bilized on SBA-15 mesoporous molecular sieve by non-covalent interactions and phosphine linkers,respectively. Both hybrid catalysts proved to be highly active and selective in cardanol metathesis andcardanol cross-metathesis with ethene and cis-1,4-diacetoxy-2-butene (DAB). GII/SBA-15 was less activethan ZC/SBA-15, however, Ru leaching was significantly lower for GII/SBA-15 (0.5%) than for ZC/SBA-15(2.5%).In ethenolysis of cardanol, 3-(non-8-enyl)phenol was isolated as a major product. In cross-metathesis with DAB 9-(3-hydroxyphenyl)non-2-enyl acetate and non-2-enyl acetate were formed withhigh selectivity. Easy catalyst?product separation and low Ru leaching provide the products (applicableas detergent precursors and fragrance and flavor agents) free from the catalyst residue.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GAP106%2F12%2F0189" target="_blank" >GAP106/12/0189: Two-dimensional zeolites with modifiable architecture</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2014

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Applied Catalysis A - General

  • ISSN

    0926-860X

  • e-ISSN

  • Volume of the periodical

    478

  • Issue of the periodical within the volume

    MAY 2014

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    8

  • Pages from-to

    138-145

  • UT code for WoS article

    000336878800017

  • EID of the result in the Scopus database