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Clustering and Photochemistry of Freon CF2Cl2 on Argon and Ice Nanoparticles

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F14%3A00429553" target="_blank" >RIV/61388955:_____/14:00429553 - isvavai.cz</a>

  • Alternative codes found

    RIV/60461373:22340/14:43897836

  • Result on the web

    <a href="http://dx.doi.org/10.1021/jp503983x" target="_blank" >http://dx.doi.org/10.1021/jp503983x</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/jp503983x" target="_blank" >10.1021/jp503983x</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Clustering and Photochemistry of Freon CF2Cl2 on Argon and Ice Nanoparticles

  • Original language description

    The photochemistry of CF2Cl2 molecules deposited on argon and ice nanoparticles was investigated. The clusters were characterized via electron ionization mass spectrometry, and the photochemistry was revealed by the Cl fragment velocity map imaging afterthe CF2Cl2 photodissociation at 193 nm. The complex molecular beam experiment was complemented by ab initio calculations. The (CF2Cl2)n clusters were generated in a coexpansion with Ar buffer gas. The photodissociation of molecules in the (CF2Cl2)n clusters yields predominantly Cl fragments with zero kinetic energy: caging. The CF2Cl2 molecules deposited on large argon clusters in a pickup experiment are highly mobile and coagulate to form the (CF2Cl2)n clusters on ArN. The photodissociation of the CF2Cl2 molecules and clusters on ArN leads to the caging of the Cl fragment. On the other hand, the CF2Cl2 molecules adsorbed on the (H2O)N ice nanoparticles do not form clusters, and no Cl fragments are observed from their photodissociation

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GA14-08937S" target="_blank" >GA14-08937S: Atmospheric Clusters and Aerosols: Molecular Beam Experiments and Theory</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2014

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Physical Chemistry A

  • ISSN

    1089-5639

  • e-ISSN

  • Volume of the periodical

    118

  • Issue of the periodical within the volume

    26

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    10

  • Pages from-to

    4740-4749

  • UT code for WoS article

    000338692800015

  • EID of the result in the Scopus database