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FT-spectroscopy of the 12C18O rare isotopologue and deperturbation analysis of the A1Π(v = 3) level

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F24%3A00584309" target="_blank" >RIV/61388955:_____/24:00584309 - isvavai.cz</a>

  • Result on the web

    <a href="https://www.sciencedirect.com/science/article/pii/S138614252400177X?via%3Dihub" target="_blank" >https://www.sciencedirect.com/science/article/pii/S138614252400177X?via%3Dihub</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.saa.2024.124011" target="_blank" >10.1016/j.saa.2024.124011</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    FT-spectroscopy of the 12C18O rare isotopologue and deperturbation analysis of the A1Π(v = 3) level

  • Original language description

    Research on 12C18O was carried out using two complementary Fourier-transform methods: (1) vacuum-ultraviolet absorption spectroscopy, with an accuracy ca. 0.03cm-1 on the DESIRS beamline (SOLEIL synchrotron) and (2) visible emission spectroscopy with an accuracy of about 0.005-0.007cm-1 by means of the Bruker IFS 125HR spectrometer (University of Rzeszow). The maximum rotational quantum number of the energy levels involved in the observed spectral lines was Jmax=54. An effective Hamiltonian and the term-value fitting approach were implemented for the precise analysis of the A1Pi(v=3) level in 12C18O. It was performed by means of the PGOPHER code. The data set consisted of 571 spectral lines belonging to the A1Pi-X1Sigma+(3, 0), B1Sigma+-A1Pi(0, 3), C1Sigma+-A1Pi(0, 3) bands and several lines involving states that perturb the A1Pi(v=3) level as well as to the previously analysed B1Sigma+-X1Sigma+(0, 0) and C1Sigma+-X1Sigma+(0, 0) transitions. A significantly extended quantum-mechanical description of the A1Pi(v=3) level in 12C18O was provided. It consists of the 5 new unimolecular interactions of the spin-orbit and rotation-electronic nature, which had not been taken into account previously in the literature. The ro-vibronic term values of the A1Pi(v=3, Jmax=55), a'3Sigma+(v=13), D1Delta(v=4) and I1Sigma-(v=5) levels were determined with precision improved by a factor of 10 relative to the previously known values.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

    <a href="/en/project/EF16_019%2F0000778" target="_blank" >EF16_019/0000778: Center for advanced applied science</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2024

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Spectrochimica Acta Part A-Molecular and Biomolecular Spectroscopy

  • ISSN

    1386-1425

  • e-ISSN

    1873-3557

  • Volume of the periodical

    312

  • Issue of the periodical within the volume

    MAY 2024

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    16

  • Pages from-to

    124011

  • UT code for WoS article

    001210219800001

  • EID of the result in the Scopus database

    2-s2.0-85186556114