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The Unexpected gas-phase reactivity of the CH3OH adduct of Michler?s hydrol blue: Proton-shuttle catalysis and stepwise radical expulsion

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388963%3A_____%2F07%3A00089489" target="_blank" >RIV/61388963:_____/07:00089489 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    The Unexpected gas-phase reactivity of the CH3OH adduct of Michler?s hydrol blue: Proton-shuttle catalysis and stepwise radical expulsion

  • Original language description

    Electrospray ionization of a methanolic solution of Michler?s hydrol blue, bis(4-(N,N-dimethylamino)phenyl)methyl tetrafluoroborate, 1+BF4?, produces the formal methanol adduct [1+ .CH3OH], which shows an unusual gas-phase chemistry. The results also question the otherwise successful kinetic method.

  • Czech name

    Neočekávaná reaktivity CH3OH aduktu Michlerovy hydrolové modři v plynné fázi: katalýza přenosem protonu a postupná eliminace radikálů

  • Czech description

    Ionizace elektrosprejem methanolového roztoku Michlerovy modři, bis(4-(N,N-dimethylamino)fenyl)methyl tetrafluoroborate, 1+BF4?, poskytuje formální methanolový adukt [1+ .CH3OH], jež má neobvyklou chemii v plynné fázi. Výsledky také zpochybňují jinak úspěšnou kinetickou metodu.

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2007

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Physical Chemistry A

  • ISSN

    1089-5639

  • e-ISSN

  • Volume of the periodical

    111

  • Issue of the periodical within the volume

    37

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    9

  • Pages from-to

    8925-8933

  • UT code for WoS article

  • EID of the result in the Scopus database