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Design, Synthesis, and Biological Evaluation of Isothiosemicarbazones with Antimycobacterial Activity

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388963%3A_____%2F17%3A00478148" target="_blank" >RIV/61388963:_____/17:00478148 - isvavai.cz</a>

  • Alternative codes found

    RIV/00216208:11160/17:10365149 RIV/00179906:_____/17:10365149 RIV/71009396:_____/17:N0000010

  • Result on the web

    <a href="http://dx.doi.org/10.1002/ardp.201700020" target="_blank" >http://dx.doi.org/10.1002/ardp.201700020</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/ardp.201700020" target="_blank" >10.1002/ardp.201700020</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Design, Synthesis, and Biological Evaluation of Isothiosemicarbazones with Antimycobacterial Activity

  • Original language description

    A series of benzaldehyde and salicylaldehyde-S-benzylisothiosemicarbazones was synthesized and tested against 12 different strains of mycobacteria, Gram-positive and Gram-negative bacteria, and the significant selectivity toward mycobacteria was proved. Twenty-eight derivatives were evaluated for the inhibition of isocitrate lyase, which is a key enzyme of the glyoxylate cycle necessary for latent tuberculosis infection, and their iron-chelating properties were investigated. Two derivatives, 5-bromosalicylaldehyde-S-(4-fluorobenzyl)-isothiosemicarbazone and salicylaldehyde-S-(4-bromobenzyl)-isothiosemicarbazone, influenced the isocitrate lyase activity and caused a better inhibition at 10 mu mol/L than 3-nitropropionic acid, a standard inhibitor. The compounds were also found to act as exogenous chelators of iron, which is an obligate cofactor for many mycobacterial enzymes. Due to their low cytotoxicity, together with the activity against isocitrate lyase and the ability to sequester iron ions, the compounds belong to potential antibiotics with the main effect on mycobacteria.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10606 - Microbiology

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2017

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Archiv der Pharmazie

  • ISSN

    0365-6233

  • e-ISSN

  • Volume of the periodical

    350

  • Issue of the periodical within the volume

    8

  • Country of publishing house

    DE - GERMANY

  • Number of pages

    12

  • Pages from-to

  • UT code for WoS article

    000406714000003

  • EID of the result in the Scopus database

    2-s2.0-85021182451