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Structure and dynamics of solvated hydrogenoxalate and oxalate anions: theoretical study

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388971%3A_____%2F16%3A00468719" target="_blank" >RIV/61388971:_____/16:00468719 - isvavai.cz</a>

  • Alternative codes found

    RIV/60076658:12110/16:43890736 RIV/60076658:12310/16:43890736

  • Result on the web

    <a href="http://dx.doi.org/10.1007/s00894-016-3075-0" target="_blank" >http://dx.doi.org/10.1007/s00894-016-3075-0</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1007/s00894-016-3075-0" target="_blank" >10.1007/s00894-016-3075-0</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Structure and dynamics of solvated hydrogenoxalate and oxalate anions: theoretical study

  • Original language description

    Hydrogenoxalate (charge - 1) and oxalate (charge - 2) anions and their solvated forms were studied by various computational techniques. Ab initio quantum chemical calculations in gas phase, in implicit solvent and microsolvated (up to 32 water molecules) environment were performed in order to explore a potential energy surface of both anions. The solvation envelope of water molecules around them and the role of water on the conformation of the anions was revealed by means of Born-Oppenheimer molecular dynamics simulations and optimization procedures. The structure of the anions was found to be dependent on the number of water molecules in the solvation shell. A subtle interplay between intramolecular and intermolecular hydrogen bonding dictates the final conformation and thus an explicit solvent model is necessary for a proper description of this phenomena.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    EE - Microbiology, virology

  • OECD FORD branch

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2016

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Molecular Modeling

  • ISSN

    1610-2940

  • e-ISSN

  • Volume of the periodical

    22

  • Issue of the periodical within the volume

    9

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    10

  • Pages from-to

  • UT code for WoS article

    000382748100015

  • EID of the result in the Scopus database

    2-s2.0-84983316459