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Versatile application of BiVO4/TiO2 S-scheme photocatalyst: Photocatalytic CO2 and Cr(VI) reduction

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388980%3A_____%2F23%3A00573863" target="_blank" >RIV/61388980:_____/23:00573863 - isvavai.cz</a>

  • Alternative codes found

    RIV/61989100:27710/23:10252621

  • Result on the web

    <a href="https://doi.org/10.1016/j.chemosphere.2023.139397" target="_blank" >https://doi.org/10.1016/j.chemosphere.2023.139397</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.chemosphere.2023.139397" target="_blank" >10.1016/j.chemosphere.2023.139397</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Versatile application of BiVO4/TiO2 S-scheme photocatalyst: Photocatalytic CO2 and Cr(VI) reduction

  • Original language description

    Herein, the synthesis, characterization, and reduction properties of 2D TiO2 aerogel powder decorated with BiVO4 (TiO2/BiVO4) were investigated for versatile applications. First, 2D TiO2 was prepared via lyophilization and subsequently modified with BiVO4 using a wet impregnation method. The morphology, structure, composition, and optical properties were evaluated using transmission electron microscopy (TEM), X-ray diffractometry (XRD), laser-induced breakdown spectroscopy (LIBS), and diffuse reflectance spectroscopy (DRS), respectively. Significantly enhanced photocurrent densities (by 3–15 times) were obtained for TiO2/BiVO4 compared to those of pure TiO2 and BiVO4. The reduction of toxic Cr(VI) to Cr(III) was assessed, including the effect of pH on overall photocatalytic efficiency. Under acidic conditions (pH ∼ 2), Cr(VI) reduction efficiency reached 100% within 2 h. For photocatalytic CO2 reduction, the highest yields of CH4 and CO were obtained using TiO2/BiVO4. A higher efficiency for both applications was achieved because of the better separation of the electron-hole pairs in TiO2/BiVO4. The excellent stability of TiO2/BiVO4 over repeated runs highlights its potential for use in versatile environmental applications. The efficiency of TiO2/BiVO4 is due to the interplay of the structure, morphology, composition, and photoelectrochemical properties that favour the material for the presented herein photocatalytic applications.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>SC</sub> - Article in a specialist periodical, which is included in the SCOPUS database

  • CEP classification

  • OECD FORD branch

    10402 - Inorganic and nuclear chemistry

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2023

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Chemosphere

  • ISSN

    0045-6535

  • e-ISSN

    1879-1298

  • Volume of the periodical

    337

  • Issue of the periodical within the volume

    OCT

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    11

  • Pages from-to

    139397

  • UT code for WoS article

  • EID of the result in the Scopus database

    2-s2.0-85164276317