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Stimuli-responsive spherical brushes based on D-galactopyranose and 2-(dimethylamino)ethyl methacrylate

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61389013%3A_____%2F14%3A00423554" target="_blank" >RIV/61389013:_____/14:00423554 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1002/mabi.201300290" target="_blank" >http://dx.doi.org/10.1002/mabi.201300290</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/mabi.201300290" target="_blank" >10.1002/mabi.201300290</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Stimuli-responsive spherical brushes based on D-galactopyranose and 2-(dimethylamino)ethyl methacrylate

  • Original language description

    Stimuli-responsive spherical brushes composed of 6-O-methacryloyl-1,2:3,4-di-O-isopropylidene-D-galactopyranose (MAIGal) and 2-(dimethylamino)ethyl methacrylate (DMAEMA) are prepared via atom transfer radical polymerization (ATRP) using cross-linked polystyrene nanoparticles covered with a thin layer of 2-(2-bromoisobutyryloxy)ethyl methacrylate (BIEM) as ATRP initiator by the ?grafting from approach. The stimuli-responsive behavior of the deprotected spherical PMAGal-b-PDMAEMA block copolymer brushes is investigated by dynamic light scattering and cryogenic transmission electron microscopy. A brush with arms containing 160 MAGal and 170 DMAEMA monomer units shows a significant contraction of the hydrodynamic radius from 20 to 70?°C at pH?=?8 with a cloud point at 40?°C, whereas no LCST is detected at pH?=?6 and 7 due to the protonation of the DMAEMA units. Aggregates occur at low temperatures and pH 8 due to intermolecular interactions between the chains of different brushes, which di

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    BO - Biophysics

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GA202%2F09%2F2078" target="_blank" >GA202/09/2078: Bioinspired nanoparticles sensitive to environment stimuli</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2014

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Macromolecular Bioscience

  • ISSN

    1616-5187

  • e-ISSN

  • Volume of the periodical

    14

  • Issue of the periodical within the volume

    1

  • Country of publishing house

    DE - GERMANY

  • Number of pages

    11

  • Pages from-to

    81-91

  • UT code for WoS article

    000330806100006

  • EID of the result in the Scopus database