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Self-assembly thermodynamics of pH-responsive amino-acid-based polymers with a nonionic surfactant

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61389013%3A_____%2F14%3A00432165" target="_blank" >RIV/61389013:_____/14:00432165 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1021/la5031262" target="_blank" >http://dx.doi.org/10.1021/la5031262</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/la5031262" target="_blank" >10.1021/la5031262</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Self-assembly thermodynamics of pH-responsive amino-acid-based polymers with a nonionic surfactant

  • Original language description

    The behavior of pH-responsive polymers poly(N-methacryloyl-l-valine) (P1), poly(N-methacryloyl-l-phenylalanine) (P2), and poly(N-methacryloylglycyne-l-leucine) (P3) has been studied in the presence of the nonionic surfactant Brij98. The pure polymers phase-separate in an acidic medium with critical pHtr values of 3.7, 5.5, and 3.4, respectively. The addition of the surfactant prevents phase separation and promotes reorganization of polymer molecules. The nature of the interaction between polymer and surfactant depends on the amino acid structure in the side chain of the polymer. This effect was investigated by dynamic light scattering, isothermal titration calorimetry, electrophoretic measurements, small-angle neutron scattering, and infrared spectroscopy. Thermodynamic analysis revealed an endothermic association reaction in P1/Brij98 mixture, whereas a strong exothermic effect was observed for P2/Brij98 and P3/Brij98. Application of regular solution theory for the analysis of experim

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CC - Organic chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/LH14292" target="_blank" >LH14292: Crosstalk between pH and temperature responsivity: How it can be used for polymer nanoparticulate systems for biomedical applications?</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2014

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Langmuir

  • ISSN

    0743-7463

  • e-ISSN

  • Volume of the periodical

    30

  • Issue of the periodical within the volume

    38

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    12

  • Pages from-to

    11307-11318

  • UT code for WoS article

    000342607000008

  • EID of the result in the Scopus database